Research on Radioactive Contaminated Soil Sorting and Volume-reducing Device
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摘要: 放射性污染场地整治及修复工作是保障核工业健康可持续发展的重要支撑。针对某典型区域放射性污染土壤的处理需求,开展源项分析和分拣机理实验,确定放射性污染土壤分拣减容工艺方案及装置设计指标,设计了一种新型放射性污染土壤分拣减容装置。该装置可实现放射性污染土壤的烘干、筛分、在线检测及按处置需求分离等功能。性能验证结果表明,其对放射性污染土壤中137Cs的理论检出限为20.7 Bq/kg,处理能力可达106 kg/h,满足设计指标。该装置有望在后续工程实施中实现某典型区域部分污染土壤从低放射性废物向极低放射性废物或极低放射性废物向免管废物的降级。本研究可为放射性污染土壤处理工作的工艺设计及工程验证提供理论指导和实验基础。Abstract: The remediation and restoration of radioactive contaminated sites has become an important support to ensure the healthy and sustainable development of the nuclear industry. In this paper, according to the treatment requirements of radioactive contaminated soil in typical areas, the source term analysis and sorting principle test are carried out to determine the radioactive contaminated soil sorting and volume-reducing process scheme and the device design indicators. Then a novel radioactive contaminated soil sorting and volume-reducing device is designed, which could realize the functions of radioactive contaminated soil drying, screening, online detection and separation according to disposal requirements. The performance verification results show that the theoretical detection limit of 137Cs in radioactive contaminated soil is 20.7 Bq/kg, and the treatment capacity can reach 106 kg/h, which meets the design indicator. The device is expected to realize the downgrade of part of the contaminated soil in a typical area from low-level radioactive waste to extremely low-level radioactive waste or extremely low-level radioactive waste to exempt waste in the follow-up project implementation. The research can provide theoretical guidance and experimental basis for the process design and engineering verification of radioactive contaminated soil treatment.
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Key words:
- Radioactive contaminated soil /
- Screening /
- Detection /
- Sorting /
- Volume-reducing
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表 1 测量时间与检出限
Table 1. Measuring Time and Detection Limit
测量时间/s MDAC/(Bq·kg−1) 137Cs 60Co 5 67.7042 63.8503 10 47.2281 44.3796 20 33.0723 30.9965 30 26.8866 25.1694 40 23.2242 21.7255 50 20.7355 19.3880 60 18.9040 17.6692 -
[1] 沈威,高柏,章艳红,等. 化学淋洗法对铀污染土壤的修复效果研究[J]. 有色金属(冶炼部分),2019(11): 81-86. [2] 谢广智,骆枫,林力,等. 放射性污染土壤修复方法概述及评价[J]. 四川环境,2018, 37(1): 164-168. doi: 10.3969/j.issn.1001-3644.2018.01.029 [3] AREVA. Japan: mapping contamination at Fukushima with robots[EB/OL]. (2013-06-20)[2021-09-20]. https://www.sa.areva.com/EN/news-9866/Japan-Mapping-contamination-at-Fukushima-with-robots.html. [4] WNN. French soil decontamination tested in Fukushima[EB/OL]. (2018-04-13)[2021-09-20]. https://www.world-nuclear-news.org/WR-French-soil-decontamination-tested-in-Fukushima-1304184.html. [5] MAYBERRY J L, FEIZOLLAHI F, DEL SIGNORE J C. Preliminary systems design study assessment report: EGG-WTD-9594 Vol. 7[R]. Butte County, Idaho: Idaho National Engineering Laboratory, 1992: 1-29. [6] 储星铭,付宸. 土壤湿度对现场γ能谱测量的影响修正[J]. 原子能科学技术,2012, 46(S1): 547-551. [7] CURRIE L A. Limits for qualitative detection and quantitative determination. Application to radiochemistry[J]. Analytical Chemistry, 1968, 40(3): 586-593. doi: 10.1021/ac60259a007 [8] 董传江, 刘莎莎, 吴耀, 等. HPGeγ谱仪放射性活度测量的刻度修正研究[C]//中国核科学技术进展报告(第六卷)——中国核学会2019年学术年会论文集第6册(核化工分卷、辐射防护分卷). 包头: 中国核学会, 2019: 348-352. [9] 谷懿. 航空伽玛能谱测量大气氡校正方法研究[D]. 成都: 成都理工大学, 2010. [10] 葛良全, 熊盛青, 曾国强, 等. 航空伽马能谱探测技术与应用[M]. 北京: 科学出版社, 2016: 116-117.